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Many laboratories are engaged in combustion research Developments in this important diagnostic area have been reviewed by Eckbreth (1988), Greenhalgh (1988), Leipertz (1989), and Stricker and Meier (1994) Combustion studies in engines include thermometry in a diesel engine (Kajiyama et al, 1982), in a production petrol engine (Greenhalgh et al, 198S), and thermometry and species measurements in a fully afterburning jet engine (Eckbreth et al, 1984) Investigations on turbulent flames were performed by Eckbreth and Hall (1 979) and on sooting flames by Hall and Boedecker (1984) as well as by Bengtsson et al (1992) Temperature information from CARS spectra derives from spectral shapes either of the @branches or of the pure rotational CARS spectra of the molecular constituents.

with part of its solvation sphere from a charged liquid surface under eld stress represents the onset of an electrohydrodynamic disintegration process on a molecular scale (29). However, Labowsky, Fenn, and de la Mora recently pointed out that the process of emission of a singly charged nanodrop from a larger drop is radically different from a Coulomb explosion, being in fact indistinguishable from Iribarne Thompson ionization (30). Such nanoscale processes (ion or nanodroplet desorption from the surface of the precursor droplet) should be facilitated by the discrete nature of the surface charge, which is shown to increase the local electrostatic pressure by at least an order of magnitude compared to the continuous charge distribution (31). Still, even though the careful analytical treatment of such processes indicates that there is a distinct possibility of small ion cluster evaporation from the charged droplet, the window of conditions that lead to ion evaporation appears to be very narrow (30). In the case of water droplets, evaporation of small ions can only occur from relatively small droplets close to the Rayleigh instability limit. The possibility of larger ion (e.g., biopolymers) desorption from electrosprayed droplets still awaits careful consideration, although the accumulated experimental evidence suggests that production of such macro-ions occurs via Dole s CRM mechanism (19, 32, 33). A very distinct feature of ESI is the accumulation of multiple charges on a single analyte molecule during ionization. Both the CRM and IEM predict accumulation of a signi cant number of charges on a macromolecule, and this

In combustion research it is most common to perform thermometry from nitrogen since it is the dominant constituent and present everywhere in large concentration despite the extent of chemical reaction The Q-branch of nitrogen changes its shape due to the increased contribution of higher rotational levels which become more populated when the temperature increases Figure 61-21 displays a calculated temperature dependence of the N2 CARS spectrum for experimental parameters typically used in CARS thermometry (Hall and Eckbreth, 1984) Note that the wavenumber scale corresponds to the absolute wavenumber value for the -2320 cni I Q-branch of N2 when excited with the frequency doubled Nd:YAG laser at 532 nm (- 18796 cm-'), i e fioT 18796 2320 = 21 116 = cm I The bands lower than about 21 I00 cm-' are due to the rotational structure of the first vibrational hot band.

For the case that there are not too many constituents in the gas under investigation the use of the pure rotational CARS technique (Zheng et al, 1984; Alden et al, 1986) may be superior to vibrational CARS thermometry since the spectra are easily resovable (for N2 the adjacent rotational peaks have a spacing of appr 8 cm I ) compared with the.

19

when the signal is at a low voltage When a # symbol is not present after the signal name, the signal is active, or asserted at the high voltage level Table H-2 Svmbol A20M# Quick Pin Reference Name and Function When the address bit 20 mask pin is asserted, the PentiumTM Processor emulates the address wraparound at one Mbyte which occurs on the 8086 When A20M# is asserted, the Pentium processor masks physical address bit 20 (A20) before performing a lookup to the internal caches or driving a memory cycle on the bus The effect of A20M# is undefined in protected mode A20M# must be asserted only when the processor is in real mode I/O As outputs, the address lines of the processor along with the byte enables define the physical area of memory or I/O accessed The external system drives the inquire address to the processor on A31-A5.

Set fs = CreateObject( Scripting.FileSystemObject ) Set f = fs.OpenTextFile(aFile, ForAppending) f.WriteLine theHeaderLine f.WriteBlankLines f.WriteLine theDataLine f.WriteBlankLines 1 f.WriteLine theFooterLine